Effective supply of reactants and product-water removal are the key issues in proton exchange membrane fuel cell (PEMFC) from the performance view point. Reactant distribution pattern can be one of the potential solutions for the well known water management problem in PEMFC. To study the effect of different flow configurations on the cell performance, three different flow-distributors, namely, parallel, serpentine, and mixed are analyzed numerically. A three-dimensional, numerical study was carried out in the three distributors for the identical reaction area. The effect of operating parameters such as flow rate and temperature was studied. The mixed flow-distributor is found to exhibit the best electrochemical performance as well as moderate pressure drop compared with the parallel and serpentine flow-distributors. The observation was confirmed by appropriate experimental study involving similar distributor geometries. Better reactant accessibility to the catalyst layer and moderate product-water removal from the cathode without diluting the reactant is argued to be the reason behind the better performance for the mixed-distributor.

1.
Ralph
,
T. R.
,
Hards
,
G. A.
,
Keating
,
J. E.
,
Campbell
,
S. A.
,
Wilkinson
,
D. P.
,
Davis
,
M.
,
St-Pierre
,
J.
, and
Johnson
,
M. C.
, 1997, “
Low Cost Electrodes for Proton Exchange Membrane Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
144
(
11
), pp.
3845
3857
.
2.
Bernardi
,
D. M.
, 1990, “
Water-Balance Calculations for Solid-Polymer-Electrolyte Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
137
(
11
), pp.
3344
3350
.
3.
Springer
,
T. E.
,
Zawodzinski
,
T. A.
, and
Gottesfeld
,
S.
, 1991, “
Polymer Electrolyte Fuel Cell Model
,”
J. Electrochem. Soc.
0013-4651,
138
, pp.
2334
2342
.
4.
Gurau
,
V.
,
Barbir
,
F.
, and
Liu
,
H.
, 2000, “
An Analytical Solution of a Half-Cell Model for PEM Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
147
, pp.
2468
2477
.
5.
Yi
,
J. S.
, and
Nguyen
,
T. V.
, 1999, “
Multicomponent Transport in Porous Electrodes of Proton Exchange Membrane Fuel Cells Using the Interdigitated Gas Distributors
,”
J. Electrochem. Soc.
0013-4651,
146
(
1
), pp.
38
45
.
6.
Rowe
,
A.
, and
Li
,
X.
, 2001, “
Mathematical Modeling of Proton Exchange Fuel Cell
,”
J. Power Sources
0378-7753,
102
, pp.
82
96
.
7.
Um
,
S.
,
Wang
,
C. Y.
, and
Chen
,
K. S.
, 2000, “
Computational Fluid Dynamics Modeling of Proton Exchange Membrane Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
147
, pp.
4485
4493
.
8.
Dutta
,
S.
,
Shimpalee
,
S.
, and
Zee
,
J. W. V.
, 2000, “
Three-Dimensional Numerical Simulation of Straight Channel PEM Fuel Cells
,”
J. Appl. Electrochem.
0021-891X,
30
, pp.
135
146
.
9.
Weber
,
A. Z.
, and
Newman
,
J.
, 2006, “
Coupled Thermal and Water Management in Polymer Electrolyte Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
153
(
12
), pp.
A2205
A2214
.
10.
Yi
,
J. S.
, and
Nguyen
,
T. V.
, 1998, “
An Along-the-Channel Model for Proton Exchange Membrane Fuel Cells
,”
J. Electrochem. Soc.
0013-4651,
145
(
4
), pp.
1149
1159
.
11.
Lee
,
J. H.
, and
Lalk
,
T. R.
, 1998, “
Modeling Fuel Cell Stack Systems
,”
J. Power Sources
0378-7753,
73
(
2
), pp.
229
241
.
12.
Ganesh Mohan
,
B.
,
Rao
,
B. P.
,
Das
,
S. K.
,
Pandiyan
,
S.
,
Rajalakshmi
,
N.
, and
Dhathathreyan
,
K. S.
, 2004, “
Analysis of Flow Maldistribution of Fuel and Oxidant in a PEMFC
,”
ASME J. Energy Resour. Technol.
0195-0738,
126
, pp.
262
270
.
13.
Slattery
,
J. C.
, and
Bird
,
R. B.
, 1958, “
Calculation of the Diffusion Coefficient of Dilute Gases and of the Self-Diffusion Coefficient of Dense Gases
,”
AIChE J.
0001-1541,
4
, pp.
137
142
.
14.
Selvarani
,
G.
,
Sahu
,
A. K.
,
Choudhury
,
N. A.
,
Sridhar
,
P.
,
Pitchumani
,
S.
, and
Shukla
,
A. K.
, 2007, “
A Phynyl-Sulfonic Acid Anchored Carbon-Supported Platinum Catalyst for Polymer Electrolyte Fuel Cell Electrodes
,”
Electrochim. Acta
0013-4686,
52
, pp.
4871
4877
.
15.
Patel
,
S.
,
Bansode
,
A. S.
,
Sundararajan
,
T.
, and
Das
,
S. K.
, 2008, “
The Performance Analysis of a Multi-Duct Proton Exchange Membrane Fuel Cell Cathode
,”
International J. Green Energy
,
5
(
1–2
), pp.
35
54
.
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